红茶加工过程香气变化研究进展

doi:10.13305/j.cnki.jts.2018.01.002

Abstract

Abstract: Aroma, as an important character of black tea, influences the intuitive judgment of tea drinkers. Black tea got various scents by the volatile compounds from glycosides hydrolyzation, carotenoids and lipids degradation, Maillard reaction pathway, and caramelization reaction. This paper reviewed the influencing factors involved in aroma formation during black tea processing from fresh tea leaves, withering, rolling, fermentation, to drying. The prospects for future research trends of black tea aroma were also suggested.

Key words: black tea, aroma, formation mechanism

CLC Number:

LIU Fei, WANG Yun, ZHANG Ting, TANG Xiaobo, WANG Xiaoping, LI Chunhua. Review on Aroma Change during Black Tea Processing[J]. Journal of Tea Science, 2018, 38(1): 9-19.

References 79

[1]	Yang Z Y, Baldermann S, Watanabe N.Recent studies of the volatile compounds in tea[J]. Food Research International, 2013, 53(2): 585-599.
[2]	吴勇. 萜烯类化合物与茶叶香气[J]. 化学工程与装备, 2009, 32(11): 123-125.
[3]	骆耀平. 茶树栽培学[M]. 4版. 北京: 中国农业出版社, 2008: 77-107.
[4]	刘声传, 曹雨, 鄢东海, 等. 贵州野生茶树资源地理分布和形态特征与气候要素的关系[J]. 茶叶科学, 2013, 33(6): 517-525.
[5]	金志凤, 叶建刚, 杨再强, 等. 浙江省茶叶生长的气候适宜性[J]. 应用生态学报, 2014, 25(4): 967-973.
[6]	徐辉, 李磊, 李庆会, 等. 大气CO2浓度与温度升高对茶树光合系统及品质成分的影响[J]. 南京农业大学学报, 2016, 39(4): 550-556.
[7]	罗凡, 龚雪蛟, 张厅, 等. 氮磷钾对春茶光合生理及氨基酸组分的影响[J]. 植物营养与肥料学报, 2015, 21(1): 147-155.
[8]	董迹芬, 边金霖,朱全武, 等. 茶叶香气与产地土壤条件的关系[J]. 浙江大学学报(农业与生命科学版), 2013, 39(3): 309-317.
[9]	Liu M, Xie F C, Cao R R, et al.Effect of different cover cultivations in later summer on aroma constituents of autumn tea (Camellia sinensis L.)[J]. Journal of Agricultural Chemistry and Environment, 2014, 3: 1-6.
[10]	张正群, 田月月, 高树文, 等. 茶园间作芳香植物罗勒和紫苏对茶园生态系统影响研究[J]. 茶叶科学, 2016, 36(4): 389-395.
[11]	陈周一琪,王志岚. 肯尼亚茶产业与茶树资源育种研究[J]. 中国农学通报, 2012, 28(19): 97-103.
[12]	王志岚, 陈亮. 印度茶树资源与育种[J]. 中国茶叶, 2011, 33(6): 4-5.
[13]	王秋霜, 乔小燕, 吴华玲, 等. 斯里兰卡五大区域红茶香气物质的HS-SPME/GC-MS研究[J]. 食品研究与开发, 2016, 37(22): 128-133.
[14]	乔小燕, 王秋霜, 陈栋. 主要产茶国茶树资源与红茶育种研究进展[J]. 植物遗传资料学报, 2015, 16(6): 1135-1140.
[15]	Yin J F, Zhang Y N, Du Q Z, et al.Effect of Ca2+ concentration on the tastes from the main chemicals in green tea infusions[J]. Food Research International, 2014, 62: 941-946.
[16]	Kelebek H.LC-DAD-ESI-MS/MS characterization of phenolic constituents in Turkish black tea: effect of infusion time and temperature[J]. Food Chemistry, 2016, 204(2): 227-238.
[17]	Xu Y Q, Zou C, Gao Y, et al.Effect of the type of brewing water on the chemical composition, sensory quality and antioxidant capacity of Chinese teas[J]. Food Chemistry, 2017, 236: 142-151.
[18]	刘盼盼, 徐勇泉, 尹军峰, 等. 主要水质因子对清香型黄山毛峰茶挥发性成分的影响[J]. 中国食品学报, 2016, 16(1): 245-257.
[19]	Schuh C, Schieberle P.Characterization of the key aroma compounds in the beverage prepared from Darjeeling black tea: quantitative differences between tea leaves and infusion[J]. Journal of Agricultural and Food Chemistry, 2006, 54(3): 916-924.
[20]	Muthumani T, Verma D P, Venkatesan S, et al.Influence of climatic seasons on quality of south Indian black teas[J]. Journal of Natural Products, 2013, 3(1): 30-39.
[21]	宁井铭, 方俊婷, 朱小元, 等. 基于代谢谱分析的祁门红茶加工过程中儿茶素及芳香类物质变化[J]. 食品工业科技, 2016, 37(9): 127-133, 138.
[22]	陈贤明, 冯林, 沈强, 等. 肯尼亚红碎茶与滇红工夫香气成分比较分析[J]. 西南师范大学学报(自然科学版), 2012, 37(7): 90-98.
[23]	Pang X L, Qin Z H, Zhao L, et al.Development of regression model to differentiate quality of black tea (Dianhong): correlate aroma properties with instrumental data using multiple linear regression analysis[J]. International Journal of Food Science and Technology, 2012, 47(11): 2372-2379.
[24]	雷攀登, 黄建琴, 丁勇, 等. 不同区域祁门红茶品质特点分析[J]. 食品科学, 2015, 36(10): 144-149.
[25]	郭雯飞, 吕毅, 江元勋. 正山小种和烟正山小种红茶的香气组成[J]. 中国茶叶加工, 2005(4): 18-23.
[26]	赖幸菲, 潘顺顺, 李裕南, 等. 不同季节和茶类的金萱品种茶叶香气成分分析[J]. 食品工业科技, 2015, 30(10): 62-68, 72.
[27]	徐元骏, 何靓, 贾玲燕, 等. 不同地区及特殊品种红茶香气的差异性[J]. 浙江大学学报(农业与生命科学版), 2015, 41(3): 323-330.
[28]	王秋霜, 吴华玲, 陈栋, 等. 广东英德红茶代表产品的香气成分鉴定研究[J]. 茶叶科学, 2012, 32(5): 448-456.
[29]	王秋霜, 乔小燕, 操君喜, 等. 广东单丛茶树品种红茶香气成分的GC-MS分析[J]. 食品科学, 2015, 36(4): 114-118.
[30]	刘晶晶, 王富民, 刘国峰, 等. 茶树萜类香气物质代谢谱与相关基因表达谱时空变化关系[J]. 园艺学报, 2014, 41(10): 2094-2016.
[31]	Mizutani M, Nakanish H, Ema J, et al.Cloning of β-primeverosidase from tea leaves: a key enzyme in tea aroma formation[J]. Plant Physiology, 2002, 130(12): 2164-2176.
[32]	夏涛, 童启庆, 董尚胜, 等. 红茶萎凋发酵中β-葡萄糖苷酶的活性变化[J]. 茶叶科学, 1996, 16(1): 63-66.
[33]	Guo W F, Yamaguchi K, Watanabe N, et al.Isolation and characterization of β-primeverosidase concerned with alcoholic aroma formation in tea leaves[J]. Bioscience, Biotechnology, and Biochemistry, 1996, 60(11): 1810-1814.
[34]	张正竹, 宛晓春, 坂田完三. 茶叶β-葡萄糖苷酶亲和层析醇化与性质研究[J]. 茶叶科学, 2005, 25(1): 16-22.
[35]	邓慧莉, 周子维, 王秋铭, 等. 武夷岩茶加工工过程β-葡萄糖苷酶对香气形成的影响[J]. 福建茶叶, 2016, (2): 1-3, 7.
[36]	陈亮, 赵丽萍, 马春雷, 等. 茶树β-葡萄糖苷酶和β-樱草糖苷酶基因表达差异分析[J]. 园艺学报, 2009, 36(1): 87-92.
[37]	周汉琛, 雷攀登, 丁勇. 茶树β-葡萄糖苷酶研究进展[J]. 茶叶科学, 2016, 36(2): 111-118.
[38]	Ohgami S, Ono E, Horikawa M, et al.Volatile glycosylation in tea plants: Sequential glycosylations for the biosynthesis of aroma β-primeverosides are catalyzed by two Camellia sinensis glycosyltransferases[J]. Plant Physiology, 2015, 168: 467-477.
[39]	Gui J D, Fu X M, Zhou Y, et al.Dose enzymatic hydrolysis of glycosidically bound volatile compounds really contribute to the formation of volatile compounds during the oolong tea manufacturing process?[J]. Journal of Agricultural and Food Chemistry, 2015, 63(31): 6905-6914.
[40]	Zhou Y, Zeng L T, Gui J D, et al.Functional characterizations of β-glucosidases involved in aroma compound formation in tea (Camellia sinensis)[J]. Food Research International, 2017, 96: 206-214.
[41]	张正竹, 宛晓春, 施兆鹏, 等. 鲜茶叶摊放过程中呼吸速率、β-葡萄糖苷酶活性、游离态香气和糖苷类香气前体含量的变化[J]. 植物生理学通讯, 2003, 39(2): 134-136.
[42]	夏涛, 童启庆, 董尚胜, 等. 红茶萎凋发酵过程中β-葡萄糖苷酶的活性变化[J]. 茶叶科学, 1996, 16(1): 63-66.
[43]	丰金玉, 刘昆言, 秦昱, 等. 红茶加工中多酚氧化酶、过氧化物酶和β-葡萄糖苷酶活性变化[J]. 农学学报, 2014, 4(11): 96-99.
[44]	夏涛, 童启庆. 冷冻萎凋对茶叶多酚氧化酶和β-葡萄糖苷酶活性的影响初探[J]. 浙江农业大学学报, 1997, 23(1): 1-6.
[45]	Muthumani T, Senthil Kumar R S. Studies on freeze-withering in black tea manufacturing[J]. Food Chemistry, 2001, 72: 319-327.
[46]	张贝贝, 艾仄宜, 曲凤风, 等. 黄光萎凋对红茶品质的影响[J]. 华中农业大学学报, 2016, 35(2): 108-114.
[47]	项丽慧, 林馥茗, 孙威江, 等. LED黄光对工夫红茶萎凋过程香气相关酶基因表达及活性的影响[J]. 茶叶科学, 2015, 35(6): 559-566.
[48]	Mahanta R K, Baruah S.Relationship between process of withering and aroma characteristics of black tea[J]. Journal of the Science of Food and Agriculture, 1989, 46: 461-468.
[49]	朱宏凯, 何华锋, 叶阳, 等. 温度对工夫红茶揉捻理化品质的影响[J]. 现代食品科技, 2017, 33(5): 1-8.
[50]	董春旺, 叶阳, 江用文, 等. 工夫红茶可视化富氧发酵机设计及试验研究[J]. 茶叶科学, 2015, 35(4): 370-376.
[51]	潘科, 冯林, 陈娟, 等. HS-SPME-GC-MS联用法分析不同通氧发酵加工工艺红茶香气成分[J]. 食品科学, 2015, 36(8): 181-186.
[52]	余露婷, 袁海波, 王伟伟, 等. 光照强度对发酵叶主要生化成分动态变化的影响[J]. 茶叶科学, 2016, 36(2): 149-159.
[53]	宋朝鹏, 高远, 武圣江, 等. 烤烟成熟过程中类胡萝卜素变化与其降解香气物质关系[J]. 中国农业科学, 2009, 42(8): 2875-2881.
[54]	Baldermann S, Kato M, Kurosawa M, et al.Functional characterization of a carotenoid cleavage dioxygenase 1 and its relation to the carotenoid accumulation and volatile emission during the floral development of Osmanthus fragrans Lour[J]. Journal of Experimental Botany, 2010, 61: 2967-2977.
[55]	Vogel J T, Tan B C, McCarty D R, et al. The Carotenoid cleavage dioxygenase 1 enzyme has broad substrate specificity, cleaving multiple carotenoids at two different bond positions[J]. Journal of Biological Chemistry, 2008, 283(17): 11364-11373.
[56]	Ilg A, Beyer P, Al-Babili S.Characterization of the rice carotenoid cleavage dioxygenase 1 reveals a novel route for geranial biosynthesis[J]. The Febs Journal, 2009, 276(3): 736-747.
[57]	Bouvier F, Suire C, Mutteer J, et al.Oxidative remodeling of chromoplast carotenoids: Identification of the carotenoid dioxygenase caccd and cszcd genes involved in crocus secondary metabolite biogenesis[J]. Plant Cell, 2003, 15(1): 47-62.
[58]	Ho C T, Zheng X, Li S M.Tea aroma formation[J]. Food Science and Human Wellness, 2015, 4: 9-27. 2003, 9: 1-6.
[59]	宛晓春. 茶叶生物化学 [M]. 3版. 北京: 中国农业出版社, 2011: 213-214.
[60]	Schwad W, Davidovich-Rikanati R, Lewinsohn E.Biosynthesis of Plant-dervived flavor compounds[J]. The Plant Journal, 2008, 54: 712-732.
[61]	Yaylayan V A.Recent advances in the chemistry of strecker degradation and Amadori rearrangement: implications to aroma and color formation[J]. Food Science and Technology Research, 2003, 9: 1-6.
[62]	Rizzi G P.The strecker degradation of amino acids: newer avenues for flavor formation[J]. Food Reviews International, 2008, 24: 416-435.
[63]	王旭, 冯涛, 庄海宁. 氨基酸对美拉德反应产物呈香特性的研究进展[J]. 中国调味, 2013, 38(7): 1-5,13.
[64]	Wang Y, Ho C T.Formation of 2,5-Dimethy-4-hydroxy-3(2H)-furanone through methylglyoxal: a Maillard reaction intermediate[J]. Journal of Agricultural and Food Chemistry, 2008, 56: 7405-7409.
[65]	Chen X M, Kitts D D.Indentification and quantification of α-dicarbonyl compounds produced in different suger-amino acid Maillard reaction model systems[J]. Food Research International, 2011, 44: 2775-2782.
[66]	Wong K H, Aziz A S, Mohamed S.Sensory aroma from Maillard reaction of individual and combinations of amino acids with glucose in acidic conditions[J]. International Journal of Food Science and Technology, 2008, 43: 1512-1519.
[67]	Adams A, De Kimpe N.Chemistry of 2-acetyl-1-pyrroline, 6-acetyl-1,2,3,4-tetrahydropyridine, 2-acetyl-2-thiazoline, and 5-acetyl-2,3-dihydro-4H-thiazine: extraordinary Maillard flavor compounds[J]. Chemical Reviews, 2006, 106(6): 2299-2319.
[68]	Wang K B, Liu F, Liu Z H, et al.Comparison of catechins and volatile compounds among different types of tea using high performance liquid chromatograph and gas chromatograph mass spectrometer[J]. Institute of Food Science and Technology, 2011, 46(7): 1406-1412.
[69]	Ho C T, Lin K, Shahidi F.Tea and tea products: chemistry and health-promoting properties [M]. CRC Press: Boca Raton, FL, 2009: 154-200.
[70]	Fu X M, Chen Y Y, Mei X, et al. Regulation of formation of volatile compounds of tea (Camellia sinensis) leaves by single light wavelength [J/OL]. Scientific Reports, 2015, 5, 16858. http://dx. Doi.org/10.1038/srep 16858.
[71]	Yang Z Y, Kobayashi E, katsuno T, et al. Characterization of volatile and non-volatile metabolites in etiolated leaves of tea (Camellia sinensis) plants in the dark[J]. Food Chemistry, 2012, 135(4): 2268-2276.
[72]	Shi J, Wang L, Ma C Y, et al.Aroma changes of black tea prepared from methyl jasmonate treated tea plants[J]. Journal of Zhejiang University-SCIENCE B (Biomedicine & Biotechnology), 2014, 15(4): 313-321.
[73]	Kraujalyte V, Pelvan E, Alasalvar C.Volatile compounds and sensory characteristics of various instant teas produced from black tea[J]. Food Chemistry, 2016, 194: 864-872.
[74]	Yang T, Zhu Y, Shao C Y, et al.Enantiomeric analysis of linalool in teas using headspace solid-phasemicroextraction with chiral gas chromatography[J]. Industrial Crop and Produces, 2016, 83: 17-23.
[75]	邵晨阳, 吕海鹏, 朱荫, 等. 不同茶类中挥发性萜类化合物的对映异构体[J]. 中国农业科学, 2017, 50(6): 1109-1125.
[76]	Zhu Y, Shao C Y, Lv H P, et al.Enantiomeric and quantitative analysis of volatile terpenoids in different teas (Camellia sinensis)[J]. Journal of Chromatography A, 2017, 1490: 177-190.
[77]	Sheibani E, Duncan S E, Kuhn D D, et al.Changes in flavor volatile composition of oolong tea after panning during tea processing[J]. Food Science & Nutrition, 2016, 4(3): 456-468.
[78]	Sine Y, José A. Sánchaez-López, Pablo M.Granitto, et al. Rapid and direct volatile compound profiling of black and green teas (Camellia sinensis) from different countries with PTR-ToF-MS[J]. Talanta, 2016, 152: 45-53.
[79]	Magagna F, Cordero C, Cagliero C, et al.Black tea volatiles fingerprinting by comprehensive two-dimensional gas chromatography-Mass spectrometry combined with high concentration capacity sample preparation techniques: Towards a fully automated sensomic assessment[J]. Food Chemistry, 2017, 225: 276-287.

Review on Aroma Change during Black Tea Processing

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